Munster singlet

Munster singlet

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while both singlet‐singlet annihilation and resonant two‐photon absorption have been discussed in the literature as candidates for pathways to primary matrix ion generation in maldi, the data presented here suggest that singlet‐singlet annihilation is the dominant mechanism for depopulating the singlet state in a matrix crystal excited at typical maldi fluences.

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Singlet-singlet annihilation in ultraviolet matrix-assisted laser

fluence data were compared with a numerical model assuming that under typical maldi fluence conditions a large fraction of molecules in the excited singlet state undergoes singlet‐singlet annihilation.

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in a separate set of experiments, the singlet lifetimes of several typical crystalline maldi matrices were determined and found to be considerably shorter than previously reported.