Deutschland singlet

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    Deutschland singlet

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    whereas triplet carbenes have been shown to insert into h2 through a two-step mechanism that at low temperature is assisted by quantum mechanical tunneling (qmt), singlet carbenes insert in concerted reactions with considerable activation barriers, and are thus unreactive towards h2 at cryogenic temperatures.

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  • Deutschland singlet

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    (p-methoxyphenyl)carbene is the first carbene that at cryogenic temperatures can be isolated in both its lowest energy singlet and triplet states.

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    this is the first example that shows that qmt can also be important for singlet carbenes inserting into dihydrogen.

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    Deutschland singlet

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Prof. Dr. W. Sander

he observed that a diphenyl carbene, matrix isolated in solid argon at cryogenic temperatures changes its spin state from triplet to singlet because of the interaction between a single methanol or water molecule by forming hydrogen bonds.

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both halogen bond donors cf3x form very strong complexes with the singlet state of dpc, but only weakly interact with triplet dpc.

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Prof. Dr. W. Sander
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Deutschland singlet

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upon annealing at higher temperatures (>10 k), the triplet is converted to the singlet; however, cooling back to 3 k does not restore the triplet.

deutschland singlet

therefore, depending on matrix temperature and irradiation conditions, matrices containing predominantly the triplet or singlet carbene can be generated.

uv (365 nm) irradiation of the system results in formation of predominantly the triplet carbene, whereas visible (450 nm) light shifts the photostationary equilibrium toward the singlet state.
of molecular hydrogen by a singlet carbene through quantum mechanical tunneling.